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Electronic structures of CeRu$_2X_2$ ($X$ = Si, Ge) in the paramagnetic phase studied by soft X-ray ARPES and hard X-ray photoelectron spectroscopy

机译:顺磁的CeRu $ _2X_2 $($ X $ = si,Ge)的电子结构   通过软X射线aRpEs和硬X射线光电子能谱研究相

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摘要

Soft and hard X-ray photoelectron spectroscopy (PES) has been performed forone of the heavy fermion system CeRu$_2$Si$_2$ and a $4f$-localized ferromagnetCeRu$_2$Ge$_2$ in the paramagnetic phase. The three-dimensional band structuresand Fermi surface (FS) shapes of CeRu$_2$Si$_2$ have been determined by softX-ray $h\nu$-dependent angle resolved photoelectron spectroscopy (ARPES). Thedifferences in the Fermi surface topology and the non-$4f$ electronicstructures between CeRu$_2$Si$_2$ and CeRu$_2$Ge$_2$ are qualitativelyexplained by the band-structure calculation for both $4f$ itinerant andlocalized models, respectively. The Ce valences in CeRu$_2X_2$ ($X$ = Si, Ge)at 20 K are quantitatively estimated by the single impurity Anderson modelcalculation, where the Ce 3d hard X-ray core-level PES and Ce 3d X-rayabsorption spectra have shown stronger hybridization and signature for thepartial $4f$ contribution to the conduction electrons in CeRu$_2$Si$_2$.
机译:软磁和硬X射线光电子能谱(PES)已在重磁子系统CeRu $ _2 $ Si $ _2 $和顺磁性相中定位的$ 4f $定位铁磁体CeRu $ _2 $ Ge $ _2 $中进行。 CeRu $ _2 $ Si $ _2 $的三维能带结构和费米表面(FS)形状已通过softX射线依赖于h \ nu $的角度分辨光电子能谱(ARPES)确定。分别通过$ 4f $流动模型和局部模型的能带结构定性地解释了CeRu $ _2 $ Si $ _2 $和CeRu $ _2 $ Ge $ _2 $之间的费米表面拓扑和非$ 4f $电子结构的差异。 。 CeRu $ _2X_2 $($ X $ = Si,Ge)在20 K处的Ce价是通过单一杂质Anderson模型计算定量估算的,其中Ce 3d硬X射线核能级PES和Ce 3d X射线吸收光谱具有在CeRu $ _2 $ Si $ _2 $中,部分$ 4f $对传导电子的贡献显示出更强的杂交和签名。

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